Saturday, 28 September 2024

BESSY II: Heterostructures for spintronics

 Spintronic devices work with spin textures caused by quantum-physical interactions. A Spanish-German collaboration has now studied graphene-cobalt-iridium heterostructures at BESSY II. The results show how two desired quantum-physical effects reinforce each other in these heterostructures. This could lead to new spintronic devices based on these materials.

Spintronics uses the spins of electrons to perform logic operations or store information. Ideally, spintronic devices could operate faster and more energy-efficiently than conventional semiconductor devices. However, it is still difficult to create and manipulate spin textures in materials.Graphene for Spintronics

Graphene, a two-dimensional honeycomb structure build by carbon atoms, is considered an interesting candidate for spintronic applications. Graphene is typically deposited on a thin film of heavy metal. At the interface between graphene and heavy metal, a strong spin-orbit coupling develops, which gives rise to different quantum effects, including a spin-orbit splitting of energy levels (Rashba effect) and a canting in the alignment of spins (Dzyaloshinskii-Moriya interaction. Especially the spin canting effectis needed to stabilise vortex-like spin textures, known as skyrmions, which are particularly suitable for spintronics.

Plus Cobalt Monolayers

Now, however, a Spanish-German team has shown that these effects are significantly enhanced when a few monolayers of the ferromagnetic element cobalt are inserted between the graphene and the heavy metal (here: iridium). The samples were grown on insulating substrates which is a necessary prerequisite for the implementation of multifunctional spintronic devices exploiting these effects.

Interactions observed

'At BESSY II, we have analysed the electronic structures at the interfaces between graphene, cobalt and iridium,' says Dr. Jaime Sánchez-Barriga, a physicist at HZB. The most important finding: contrary to expectations, the graphene interacts not only with the cobalt, but also through the cobalt with the iridium. 'The interaction between the graphene and the heavy metal iridium is mediated by the ferromagnetic cobalt layer,' Sánchez-Barriga explains. The ferromagnetic layer enhances the splitting of the energy levels. 'We can influence the spin-canting effect by the number of cobalt monolayers; three monolayers are best,' says Sanchez-Barriga.

This result is supported not only by experimental data, but also by new calculations using density functional theory. The fact that both quantum effects influence and reinforce each other is new and unexpected.

Source : ScienceDaily

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